Also remember that front drive lines are not always balanced and with a CV joint (which is recommended with a dual case setup), and are greatly affected by suspension lift. Despite using 2WD with the hubs engaged, if there is no torque transmitting through the line its possible to not bind, shake and rattle, which may yield a false diagnosis.
To be absolutely sure it isn't the front drive line, its best to just remove it all together and then drive in 2WD with the hubs engaged.
Mike